Viscoelastic studies on thermoplastic polyurethane nanocomposites using a nano- hardness tester

 

 

Ivan Rivera, Darren Martin, and Rowan Truss*

 

School of Engineering

The University of Queensland

Brisbane, Queensland, Australia 4072

 

 

Abstract

 

      The viscoelastic behaviour of a range of polyurethane thermoplastic elastomer montmorillonite nanocomposites has been studied using a nanohardness tester. For softer Shore hardness 80A materials, the introduction of the organo-clay increased the creep strain obtained while the nano-indentor was held at constant load. The increase in creep strain was greatest for materials containing an organo-clay modified with a more hydrophilic quaternary alkylammonium surfactant and with higher loadings of the hydrophilic organo-clay. This suggested the effect might be due to a plasticising effect of the excess surfactant. For the harder Shore hardness 55D materials, the addition of the organo-clays produced only a small decrease in the creep strain, probably due to the interconnected hard domains in this material.

 



* Corresponding author

E-mail: Rowan Truss R.Truss@uq.edu.au, Fax: +61 7 33653888